Solid solutions between BaTiO₃ and LaFeO3 have been prepared through a solid state reaction method. The X-ray diffraction results reveal that Ba_1-xLa_xTi_1-xFe_xO₃ (0.1 ≤ x ≤ 0.7) compounds have a cubic structure, whereas the parent material BaTiO₃ has a tetragonal structure. The magnetization measurements indicate that the materials have a magnetic ordering at room temperature and the magnetic properties of the solid solutions depending on the doping amount of LaFeO₃. The origin of magnetic behaviors is believed to be from Fe ³⁺ ions.